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Gregor Jotzu: Ultrafast Magnetometry of (Light-Induced) Superconductors

Driving certain cuprates and organic materials has been shown to induce THz optical properties reminiscent of superconductivity far above the equilibrium transition temperature. However, the magnetic response of these non-equilibrium states remains unexplored. This study investigates whether these states exhibit a Meissner effect, expelling external magnetic fields, and examines their response to changing magnetic fields on sub-picosecond time scales.Our methodology involves studying the ultrafast magnetic response of these materials in static and time-dependent magnetic fields using the Faraday effect in a magneto-optical crystal adjacent to the sample. This provides sub-picosecond time resolution for reconstructing the position-dependent magnetic properties.

Andrei Shumilin: Emergent spin phenomena from hyperfine interaction ‌of localized electrons and nuclear spins

Many modern devices are based on the operations with spins. They require the preparation of the initial state: with spin polarization or at least with spin correlations. There is a limited number of conventional methods to achieve this: application of ferromagnetic materials, current to spin conversion due to spin-orbit interaction and static polarization in high magnetic fields. We show the existence of another way to achieve spin polarization in non-magnetic solid-state devices. It requires small magnetic fields, hyperfine interaction between electron and nuclear spins and small exchange interaction between electron spins. All the interaction energies are considered small compared to temperature, but the mechanism requires non-equilibrium conditions.

Madhumita Sarkar: Manipulating exciton binding by floquet engineering ‌in Fermi Hubbard ladder

Strong excitations of correlated quantum materials give rise to various non-thermal phases which are not present in their equilibrium counterpart. Recently, it was shown that the one-dimensional Fermi Hubbard Model features charge density wave and η-pairing phases upon photo-doping. In this study, we explore the non-equilibrium behavior of the Fermi Hubbard ladder and employ the Schrieffer-Wolff transformation to map it to a simplified t-J-like model, providing an effective equilibrium description of the photo-doped states. Our investigation highlights the significance of applying an electric field along the rung to the hopping term. This floquet manipulation allows to increase the spin and η-exchange coupling along the rung independent of the hopping term. Moreover, the magnitude of hopping decreases as a result of the drive. These combined effect tends to localize the excitons close to each other and thus enhance its binding energy. To characterize the ground state of the system, we employ relevant correlators and make notable observations. We show that at certain drive frequencies, the ground state encompasses a strongly bound holon-holon/doublon-holon pair along the rung, alongside inter-chain singlets. Additionally, we propose experimental setups to test our theory.

Jaka Strohsack: Influence of Metal/Organic-Molecules Interface on Magnetic Anisotropy ‌in Co Thin Films: A Time-Resolved MOKE Investigation

We investigated by means of the ultrafast time-resolved magneto-optical Kerr effect (MOKE) spectroscopy the effect of the interface between organic molecular semiconductors and cobalt on the magnetic anisotropy of polycrystalline Co thin films. Comparison of the effect was measured on interfaces of Co with: nonmagnetic metal (Al), metalorganic complexes tris(8-hydroxyquinoline)gallium (Gaq3) and M-phthalocyanines (M=Cu, Co) as well as Buckminster-fullerene (C60) molecules.In general, the transient MOKE signals were found to exhibit damped coherent spin wave oscillations (CSWO) with frequencies up to several tens of GHz. Detailed analysis of the spin-wave temperature and magnetic field dependences allowed us to compare the influence of different molecular interfaces.

Dinner

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Denis Golez: Chirped amplitude mode in photo-doped superconductors

When a continuous symmetry is spontaneously broken, two types of collective modes emerge: phase and amplitude mode fluctuations of the order parameter. The latter is a massive excitation living at the edge of the gap. Recently, signatures of the amplitude mode were observed in photo-doped superconductors using third-harmonics generation in the terahertz regime, which opened the field of nonlinear light-amplitude mode coupling.We will show that a weak photo-excitation in superconductors leads to a long-lived prethermal phase with a reduced order parameter and superimposed amplitude oscillations. As we increase the intensity of the pump pulse, the amplitude mode oscillations exhibit chirping; namely, the frequency slows down as a function of time. The chirping gets amplified as we approach the nonthermal critical point - an excitation at which the intensity of the light is large enough to destroy the superconducting order. We identify signatures of the chirped amplitude mode in photo-induced current after a monocycle or Gaussian pulse and propose a transmission line circuit experiment to detect the phenomena. In the last part, we will present recent theoretical advances based on the compressed representation of quantum propagators, which allow the analysis of time scales relevant for the collective mode dynamics.

Carlo Vanoni: A renormalization group analysis of the Anderson model ‌in infinite dimensions

In this talk, I will present a renormalization group analysis of the problem of Anderson localization on Regular Random Graphs (RRGs). I will first review and extend the finite-dimensional analysis of Abrahams, Anderson, Licciardello, and Ramakrishnan in terms of spectral observables, and discuss how to take the large-d limit. I will then motivate that the infinite-dimensional case, relevant also in the context of Many-Body Localization, recovers the Anderson model on RRGs. In this case, the renormalization group β-function necessarily involves two parameters, but the one-parameter scaling hypothesis is recovered for sufficiently large system sizes. I will also discuss how to understand this change in behavior in terms of the geometrical properties of the graphs. The talk will be based on arXiv:2306.14965 and ongoing work

Rafał Świętek: A note on weak eigenstate thermalization and normalization of operators

While the eigenstate thermalization hypothesis (ETH) is well established for quantum-chaotic interacting systems, its validity for other classes of systems remains a matter of intense debate. Focusing on quadratic fermionic Hamiltonians, we here argue that the weak ETH is satisfied for few-body observables in many-body eigenstates of quantum-chaotic quadratic (QCQ) Hamiltonians. In contrast, the weak ETH is violated in two cases: (a) for sums of few-body observables in all quadratic Hamiltonians, and (b) for few-body observables in localized quadratic Hamiltonians. We argue that these properties can be traced back to the validity of single-particle eigenstate thermalization, and we highlight the subtle role of normalization of operators. Our results suggest that the difference between weak and no ETH in many-body eigenstates allows for a distinction between single-particle quantum chaos and localization. We test to which degree this phenomenology holds true for integrable systems such as the XYZ and XXZ models.

Andrew George Green: Phase Transitions in the Classical Simulability of Open Quantum Systems

We introduce a Langevin unravelling of the density matrix evolution of an open quantum system over matrix product states, which we term the time-dependent variational principle-Langevin equation. This allows the study of entanglement dynamics as a function of both temperature and coupling to the environment. As the strength of coupling to and temperature of the environment is increased, we find a transition where the entanglement of the individual trajectories saturates, permitting a classical simulation of the system for all times. This is the Hamiltonian open system counterpart of the saturation in entanglement found in random circuits with projective or weak measurements. If a system is open, there is a limit to the advantage in simulating its behaviour on a quantum computer, even when that evolution harbours important quantum effects. Moreover, if a quantum simulator is in this phase, it cannot simulate with quantum advantage.

Till Domröse: Light-induced hexatic state observed by ultrafast nanobeam diffraction

Quantum materials are characterised by enhanced correlations between their microscopic degrees of freedom that favor the occurence of exciting physical properties that are tunable by optical excitation, including the formation of charge-density waves (CDWs). The investigation of the dynamics following such an optical quench is available in ultrafast transmission electron microscopes (UTEMs), versatile tools that combine nanometer spatial with femtosecond temporal resolution (Fig. 1a).Here, we investigate the transformation between the nearly-commensurate (NC) and the incommensurate (IC) CDW phase in the layered quantum material 1T-TaS2. Therein, selective contrast enhancement by means of ultrafast dark-field microscopy allows us to follow the spatially heterogeneous suppression of the NC phase on the nanoscale, particularly at interphase boundaries. In a complementary approach, the establishment of three-dimensional IC CDW order is accessible by means of ultrafast electron diffraction. Specifically, the high-coherence electron source of the Göttingen UTEM enables collimated diffractive probing of nanometer-sized, spatially homogenous sample regions with high reciprocal-space resolution (Fig. 1c).

Anze Mraz: Switching of the nanocryotron-driven ‌charge configuration memristor in real time

To improve the field of superconducting computer systems, a low-power, fast and durable memory device that is compatible with the single-flux-quantum (SFQ) logic is needed. Here we report on recent progress in the development of a so-called parallelotron (pTron) device that comprises a superconducting three-terminal amplifying nanowire cryotron (nTron) and a charge configuration memristor (CCM) based on 1T-TaS2. Besides the current-voltage characteristics and read operation, we also record switching of the device in real time when the switching pulse is applied to the control terminal. Measured results show great matching to model predictions, demonstrating the validity of the model and its potential usefulness for future optimization of the device’s parameters. We briefly discuss the effect of noise on the switching capabilities of the pTron device.

Tomaz Mertelj: Unconventional photo-induced charge-density-wave dynamics ‌in 2H-NbSe2 compared to the conventional in 1T-VSe2

We investigated temperature dependent ultrafast near-infrared transient reflectivity dynamics in coexisting superconducting (SC) and charge density wave (CDW) phases of layered 2H-NbSe2 using NIR and visible excitations. With visible pump-photon excitation (400 nm) we find a slow high-energy quasiparticle relaxation channel which is present in all phases. In the CDW phase, we observe a distinctive transient response component. The component is marked by the absence of coherent amplitude mode oscillations and a relatively slow, picosecond rise time, which is different than in most of the typical CDW materials, such as 1T-VSe2. In the SC phase, another tiny component emerges that is associated with optical suppression of the SC phase. The transient reflectivity relaxation in the CDW phase is dominated by phonon diffusive processes with an estimated low-T heat diffusion constant anisotropy of ∼ 30. Strong excitation of the CDW phase reveals a weakly non-thermal CDW order parameter (OP) suppression. Unlike CDW systems with a larger gap, where the optical OP suppression involves only a small fraction of phonon degrees of freedom, the OP suppression in 2H-NbSe2 is characterized by the excitation of a large number of phonon degrees of freedom and significantly slower dynamics.

Manuel Tuniz: Manipulation of the charge-density-wave in VTe2 ‌by femtosecond light pulses

By combining time and angle-resolved photoemission spectroscopy (tr-ARPES) and broadband time-resolved optical spectroscopy (TR-OS) we investigate the effect of an optical excitation on the electronic and structural properties of the charge-density wave (CDW) system VTe2. Recently, the modification of the material’s electronic structure induced by CDW formation has been discussed because the strongly orbital-dependent changes may give rise to a topological change in specific bands.In our contribution, we show by means of TR-OS measurements the possibility to optically excite the amplitude mode (AM) of the CDW phase and therefore couple to the CDW condensate. Moreover, by studying the partial closing of the CDW gap our tr-ARPES experiments unveil a major role played by the lattice degrees of freedom in the stabilization of the CDW phase in VTe2.

Iris Ulčakar: Iterative construction of conserved quantities ‌in dissipative nearly integrable systems

Integrable systems offer rare examples of solvable many-body problems in the quantum world. Due to the fine-tuned structure, their realization in nature and experiment is never completely accurate, therefore effects of integrability are observed only transiently. One way to surpass that is to couple nearly integrable systems to baths and driving: these will stabilize integrable effects up to arbitrary time, as encoded in the time dependent, and eventually, the stationary state of form of a generalized Gibbs ensemble. However, the description of such driven dissipative nearly integrable models is challenging and no exact analytical methods have been proposed so far. Here we develop an iterative scheme in which integrability breaking perturbations (baths) determine the most necessary conserved quantities to be added into a truncated generalized Gibbs ensemble description. Our scheme significantly reduces the complexity of the problem, paving the way for thermodynamic results.

Jože Gašperlin: The interplay of lattice dynamics, stacking effects and Mott physics ‌in charge-density-wave systems

The transition metal dichalcogenide 1T-TaS2 is a layered compound that exhibits a series of increasingly commensurate charge density wave phases with decreasing temperature, including a low-temperature insulating phase. For a single 1T-TaS2 layer, with an odd number of electrons per Star-of-David cluster, the insulating behaviour may be attributed to Mott localisation. However, the stacking arrangement of multiple layers can lead to doubling of the unit cell, where the nature of the insulating state is ambiguous. Furthermore, the various possible stacking terminations lead to surface states with non-trivial interplay between band-insulating and Mott-insulating behaviour.

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